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Explore a groundbreaking approach to nanomaterials synthesis and engineering in this Fred Kavli Distinguished Lectureship delivered at the 2015 MRS Spring Meeting. Discover how mechanical compressive force can induce structural phase transitions in nanoparticles, enabling the creation of new nanomaterials with precisely controlled structures and tunable properties. Learn about the Stress-Induced Fabrication method, which offers a flexible alternative to traditional crystallization processes for materials engineering. Understand how manipulating nanoparticle coupling through external pressure allows for reversible changes in assemblies and properties, as well as the formation of one- to three-dimensional nanostructures. Gain insights into the potential applications and advantages of this innovative technique in the field of nanoscience.